Electrocatalytic hydrogen evolution reaction with metallophthalocyanines modified with click electrochemistry
By Duygu Aky
Published in International Journal of Hydrogen Energy
NULL
2015
Abstract
Cobalt and zinc phthalocyanines bearing terminal alkyne groups (TA-CoPc and TA-ZnPc) were electrochemically characterized in order to determine their functionalities for practical usages as effective electrocatalysts. Observation of multi-electron and metal and/or ring based reduction reactions at low potentials indicated the worthy of these complexes as functional materials. Shifts of proton reduction potentials toward more positive values in solutions involving \MPc\ indicated homogeneous electrocatalytic activities of the complexes for hydrogen evolution reaction (HER). For practical usage as heterogeneous electrocatalysts for HER, electrodes were constructed with a new electrode modification technique,
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