Bespoke Photoreductants: Tungsten Arylisocyanides
By Sattler, Wesley; Henling, Lawrence M.; Winkler, Jay R. & Gray, Harry B.
Published in Journal of the American Chemical Society
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2015
Abstract
Modular syntheses of oligoarylisocyanide ligands that are derivatives of 2,6-diisopropylphenyl isocyanide (CNdipp) have been developed; tungsten complexes incorporating these oligoarylisocyanide ligands exhibit intense metal-to-ligand charge-transfer visible absorptions that are red-shifted and more intense than those of the parent W(CNdipp)6 complex. Additionally, these W(CNAr)6 complexes have enhanced excited-state properties, including longer lifetimes and very high quant
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