Metal-Assisted Ligand-Centered Electrocatalytic Hydrogen Evolution upon Reduction of a Bis(thiosemicarbazonato)Cu(II) Complex
By Haddad, Andrew Z.; Cronin, Steve P.; Mashuta, Mark S.; Buchanan, Robert M.; Grapperhaus, Craig A.
Published in Inorganic Chemistry
2017
Abstract
In this study, we report the electrocatalytic behavior of the neutral, monomeric Cu(II) complex of diacetyl-bis(N-4-methyl-3-thiosemicarbazonato), CuL1, for metal-assisted ligand-centered hydrogen evolution in acetonitrile and dimethylformamide. CuL1 displays a maximum turnover frequency (TOF) of 10 000 s
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