[FeFe]-Hydrogenase H-Cluster Mimics with Various ?S(CH2)nS
By Abul-Futouh, Hassan; Almazahreh, Laith R.; Harb, Mohammad Kamal; G
Published in Inorganic Chemistry
2017
Abstract
The effect of the nature of the dithiolato ligand on the physical and electrochemical properties of synthetic H-cluster mimics of the [FeFe]-hydrogenase is still of significant concern. In this report we describe the cyclization of various alkanedithiols to afford cyclic disulfide, tetrasulfide, and hexasulfide compounds. The latter compounds were used as proligands for the synthesis of a series of [FeFe]-hydrogenase H-cluster mimics having the general formulas [Fe2(CO)6?-S(CH2)nS] (n = 4
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