Mechanistic Insights into the Enhanced Activity and Stability of Agglomerated Cu Nanocrystals for the Electrochemical Reduction of Carbon Dioxide to n-Propanol
By Dan Ren and Nian Tee Wong and Albertus Denny Handoko and Yun Huang and Boon Siang Yeo
Published in The Journal of Physical Chemistry Letters
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2016
Abstract
The reduction of carbon dioxide (CO2) to n-propanol (CH3CH2CH2OH) using renewable electricity is a potentially sustainable route to the production of this valuable engine fuel. In this study, we report that agglomerates of ?15 nm sized copper nanocrystals exhibited unprecedented catalytic activity for this electrochemical reaction in aqueous 0.1 M KHCO3. The onset potential for the formation of n-propanol was 200
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