Control of the substituent at the nitrogen atom in a 2,4,6-triphenylpyridinium perchlorates tunes the electrocatalytic hydrogen evolution mechanism and efficiency
By Dolganov, A. V.; Chernyaeva, O. Y.; Kostryukov, S. G.; Balandina, A. V.; Solovyova, E. O.; Yudina, A. D.; Akhmatova, A. A.; Lyukshina, Y. I.
Published in International Journal of Hydrogen Energy
2019
Abstract
Electrochemical properties and electrocatalytic activity in of hydrogen evolution reaction (HER) in new members of the family of homogeneous organic metal-free catalysts based on N-methyl and N-phenyl - 2,4,6-triphenylpyridinium perchlorates were studied using electrochemical methods. With a similar structure and electrochemical properties, the electrocatalytic behavior differs dramatically. The main reason for this is the
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